A widely used method for estimating fine scale long-term spatial variation in air pollution, especially for epidemiology studies, is land use regression (LUR) modeling using fixed off-road monitors. More recently, LUR models have been developed using data from mobile monitors that repeatedly measure road pollutants and mixed-effects modeling. Here, nitrogen dioxide (NO₂) and black carbon (BC) predictions from two independent models were compared across streets (defined as 30–60 m road segments) (N = 30,312) and residences (N = 76,752) in Copenhagen, Denmark. The first model was Google Street View (GSV)-based mixed-effects LUR models (Google-MM) that predicted 2019 mean NO₂ and BC levels, and the second was European-wide (EUW) LUR models that predicted annual mean 2010 levels at 100 m spatial resolution. Across street segments, the Spearman correlation coefficient between the 2019 NO₂ from Google-MM-LUR and 2010 NO₂ from EUW-LUR was 0.66, while at residences, this was 0.60. For BC, these were 0.51 across street segments and 0.40 at the residential level. The ratio of percentile 97.5 to 2.5 for NO₂ across the study area streets using Google-MM NO₂ was 4.5, while using EUW-LUR, this was 2.1. These NO₂ ratios at residences were 3.1 using Google-MM LUR, and 1.7 using EUW-LUR. Such ratios for BC across street segments were 3.4 using Google-MM LUR and 2.3 using EUW-LUR, while at the residential level, they were 2.4 and 1.9, respectively. In conclusion, Google-MM-LUR NO₂ for 2019 was moderately correlated with EUW-LUR NO₂ developed in 2010 across Copenhagen street segments and residences. For BC, while Google-MM-LUR was moderately correlated with EUW-LUR across Copenhagen streets, the correlation was lower at the residential level. Overall, Google-MM-LUR revealed larger spatial contrasts than EUW-LUR.