The escalating climate crisis requires rapid action to reduce the concentrations of atmospheric greenhouse gases and lower global surface temperatures. Methane will play a critical role in near-term warming due to its high radiative forcing and short atmospheric lifetime. Methane emissions have accelerated in recent years, and there is significant risk and uncertainty associated with the future growth in natural emissions. The largest natural sink of methane occurs through oxidation reactions with atmospheric hydroxyl and chlorine radicals. Enhanced atmospheric oxidation could be a potential approach to remove atmospheric methane. One method proposes the addition of iron salt aerosol (ISA) to the atmosphere, mimicking a natural process proposed to occur when mineral dust mixes with chloride from sea spray to form iron chlorides, which are photolyzed by sunlight to produce chlorine radicals. Under the right conditions, lofting ISA into the atmosphere could potentially reduce atmospheric methane concentrations and lower global surface temperatures. Recognizing that potential atmospheric methane removal must only be considered an additive measure – in addition to, not replacing, crucial anthropogenic greenhouse gas emission reductions and carbon dioxide removal – roadmaps can be a valuable tool to organize and streamline interdisciplinary and multifaceted research to efficiently move towards understanding whether an approach may be viable and socially acceptable or if it is nonviable and further research should be deprioritized. Here we present a 5-year research roadmap to explore whether ISA enhancement of the chlorine radical sink could be a viable and socially acceptable atmospheric methane removal approach.